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Contents
6
About the Authors
8
Abstract
10
1 Introduction
11
1.1 Organic Photovoltaics: Background
11
1.2 Materials: Conjugated Polymers
12
1.3 Operation Principles and Physical Insights in Organic Solar Cells (OSCs)
13
1.4 Organic Solar Cell Architectures
16
1.5 State-of-the-Art, Challenges and Opportunities in OSCs
19
1.6 Surface Plasmons for Improving Light Harvesting Efficiency
20
1.7 Other Contributions to Organic Photovoltaic Performance Improvement
25
1.8 State-of-the-Art and Challenges in Plasmonic Organic Solar Cells
26
References
27
2 Surface Plasmon Resonance
34
2.1 Introduction
34
2.2 Surface Plasmon Polariton
34
2.3 Localized Surface Plasmon Resonance
37
2.4 Summary
39
References
39
3 Characterization Plasmonic Organic Photovoltaic Devices
41
3.1 Introduction
41
3.2 Optical Spectroscopy
41
3.2.1 Steady-State and Transient Absorption Spectroscopies
41
3.2.2 Time-Integrated Photoluminescence and Time-Resolved Photoluminescence
45
3.2.3 Spatially Resolved Spectroscopy
47
3.3 Electrical Characterization
47
3.3.1 Current Voltage (I-V) Measurement
47
3.3.2 Internal Photon to Current Efficiency (IPCE) Measurement
48
3.4 Numerical Simulation
48
3.4.1 Optical Simulation
49
3.4.2 Electrical Simulation
50
3.5 Summary
53
References
54
4 Plasmonic Entities within the Charge Transporting Layer
55
4.1 Introduction
55
4.2 Case Study (1): Silver Nano-Triangle Arrays in PEDOT:PSS
57
4.3 Case Study (2): Gold Nanowire Network in PEDOT:PSS
66
4.4 Case Study (3): Single Silver Nanowire in PEDOT:PSS
75
4.5 Summary and Conclusions
84
References
84
5 Plasmonic Entities within the Active Layer
89
5.1 Introduction
89
5.2 Experimental Details
91
5.3 Results and Discussion
92
5.4 Summary and Conclusions
106
References
106
6 Concluding Remarks
109
6.1 Implications for the Design of Hybrid Plasmonic OPV Devices
109
6.2 Summary and Outlook
110
References
113
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